Aluminum based spent nuclear fuel (Al-SNF) will be treated and then stored in a geological repository. A series of corrosion tests, including coupon, galvanic, and electrochemical, were performed to measure the effects of degradation on U-Al alloys, which simulated various Al-SNF forms. The test solutions were variants of a J- 13 well water chemistry. As part of the degradation characteristics, the dissolution of uranium, which is the primary radionuclide, was measured. The degradation and dissolution were changed by the type of water chemistry and the temperature. The alloy composition and fabrication were not significant variables.